ENVIRONMENTAL PRINT (Print & Word Awareness Activity) - I Spy Letters:: Use real life items and put on a wall. I used to also have kids bring them in and put them in a photo album in the class library.
This site has TONS of resources for structured play, beginning literacy activities, and hand-eye coordination broken down by age from birth and through school years. Stoplight Beanbag Toss - I Can Teach My Child! I own bean bags already!